When did relations between the settlers and the Powhatan people improve?

The relations have improved after John Wolfe was married to the daughter of the Powhatan chief - Pocahontas

Explanation:

After the first colonists and settlers came to the Jamestown they had bad relations with the Natives. In addition to that colonists had problems with lack of food, with climate and with many other problems. This started changing after 1610 when a new group of settlers came. Finally after the marriage that was signed 1614 peace was established for some longer period of time.

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